The GREENCAP project is dedicated on developing high-performance and sustainable supercapacitors by applying the principles of green chemistry. The project targets cylindrical supercapacitor designs that incorporate advanced layered two-dimensional materials—such as graphene and MXenes—as electrode materials, along with ionic liquids as high-voltage electrolytes. This innovative approach aims to create environmentally friendly, efficient, and durable energy-storage devices for next-generation applications.
Funding: European Union
Project Duration: 01/2023-12/2025
Supercapacitors
Schematic representation of how an electrochemical double-layer capacitor (EDLC) works
Picture: Lukas Köps"Supercapacitors" are the class of electrochemical energy storage devices that store charge through a physical process. Supercapacitors are known for their high power density (>10 kW kg⁻¹ ) , rapid charge/discharge (within seconds to minutes), extended lifetime (>10⁵ cycles ), and wide operating temperature range (-40 °C to +65 °C), offering excellent safety. Nevertheless, their energy density remains significantly lower than that of lithium-ion batteries, highlighting the classic trade-off between energy and power
One key strategy to enhance energy density is to increase the device's operating voltage, as energy scales with the square of the voltage (E = 1/2 CV² ) . This requires the development of electrolytes with enhanced voltage stability, particularly above 2.8 V. Our group is actively working on developing novel ionic liquid (IL)-based electrolytes to meet this challenge.
In parallel, we are exploring sustainable approaches for next-generation EDLCs. This includes developing eco-friendly electrode materials and biomass-derived solvents such as gamma-valerolactone (GVL), which offer reduced environmental impact and improved sustainability in energy storage systems.
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Publications
Gaško, M., Patil, F.I., Köps, L., Krüger, D., Neumann, C., Turchanin, A., Kreth, F.A., and Balducci, A.; Tetraethylammonium Perfluorobutanesulfonate as an Alternative Salt for Electric Double Layer Capacitors. Batteries & Supercaps 2024, 7 (11), e202400283.
Köps, L., Kreth, F.A., Leistenschneider, D., Schutjajew, K., Gläßner, R., Oschatz, M., and Balducci, A.; Improving the stability of supercapacitors at high voltages and high temperatures by the implementation of ethyl isopropyl sulfone as electrolyte solvent. Advanced Energy Materials 2023, 13 (5), 2203821.
Köps, L., Kreth, F.A., Bothe, A., and Balducci, A.; High voltage electrochemical capacitors operating at elevated temperature based on 1,1-dimethylpyrrolidinium tetrafluoroborate. Energy Storage Materials 2022, 44, 66-72.
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Orbay, Metin Taha, Dr Postdoc, Project: GREENCAP Professorship of Applied Electrochemistry
Room R 129
Humboldtstraße 8
07743 Jena
Image: Desirée Leistenschneider -
Patil, Indrajit Mahadev, Dr Postdoc, Project: GREENCAP Professorship of Applied Electrochemistry
Room R 129
Humboldtstraße 8
07743 JenaImage: Anne Günther (University of Jena) -
Fatima, Urooj PhD Student, Project: ENERCAP Professorship of Applied Electrochemistry
Room R 127
Lessingstraße 14
07743 Jena
Image: Desirée Leistenschneider -
Kost, Rebecka PhD Student, Project: EXTREME Professorship of Applied Electrochemistry
Room R 127
Lessingstraße 14
07743 Jena
Image: Desirée Leistenschneider -
Nowacki, Bartosz Pawel PhD Student, Project: ENERCAP Professorship of Applied Electrochemistry
Room R 127
Lessingstraße 14
07743 Jena
Image: Desirée Leistenschneider